This data release includes raw detrital zircon U-Pb data for Paleoproterozoic metasedimentary rocks of the Gunnison block, central Colorado, USA. Detrital zircon U-Pb data for five samples of metasedimentary rock (totaling 1459 zircon U-Pb dates) were acquired via laser ablation-inductively coupled plasma-mass spectrometry (LA-ICP-MS) at the University of Arizona LaserChron Center. The data provide constraints on the sediment provenance, maximum depositional age, and timing of metamorphism of these metasedimentary rocks, providing insights on the crustal and tectonic evolution of the Gunnison block and Yavapai Province.