Plume-scale testing of a simplified method for detecting tritium contamination in plants and soil

Cost-effective methods are needed to detect contamination near radioactive-waste and other contaminated sites. Such methods should be capable of providing an early warning of contaminant releases and should be accurate and robust enough for assessing the long-term performance of waste-isolation facilities and remediation measures. Recently, a simplified method for detecting tritium contamination in plants and soil was developed (1). The method includes solar distillation of plant water from foliage, followed by filtration and adsorption of scintillation-interfering constituents on a graphite-based solid-phase-extraction column prior to direct-scintillation counting. The objectives of the in-progress study described here are to (i) test the simplified contamination-detection method for collection and analysis of plume-scale tritium data and (ii) gain insight into tritium migration pathways and processes.